In article number 1801955, Hangxun Xu, Yujie Xiong, and co‐workers highlight the recent advances in the development of photocatalysts based on two‐dimensional polymer nanosheets for photocatalytic overall water splitting, with a focus on tuning their electronic structures and surface active sites. Such two‐dimensional polymer nanosheets can convert solar energy into chemical fuels due to their tunable electronic and optical properties.
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