The design and synthesis of lightweight and strong materials are essential for developing next‐generation structural materials. In article number 1802997, Seok Joon Kwon, Pil J. Yoo, and co‐workers demonstrate a new class of graphene‐based, ultralight, strong, and superelastic closed‐cellular structures by developing an innovative hierarchical architecturing strategy. The achieved structure is a uniformly ordered plesiohedral cellular structure with complete space‐filling convex polytopes.
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